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TitleRevealing energy level structure of individual quantum dots by tunneling rate measured by single-electron sensitive electrostatic force spectroscopy.
Publication TypeJournal Article
Year of Publication2015
AuthorsRoy-Gobeil, Antoine, Yoichi Miyahara, and Peter Grutter
JournalNano Lett
Volume15
Issue4
Pagination2324-8
Date Published2015 Apr 8
ISSN1530-6992
Abstract

We present theoretical and experimental studies of the effect of the density of states of a quantum dot (QD) on the rate of single-electron tunneling that can be directly measured by electrostatic force microscopy (e-EFM) experiments. In e-EFM, the motion of a biased atomic force microscope cantilever tip modulates the charge state of a QD in the Coulomb blockade regime. The charge dynamics of the dot, which is detected through its back-action on the capacitavely coupled cantilever, depends on the tunneling rate of the QD to a back-electrode. The density of states of the QD can therefore be measured through its effect on the energy dependence of tunneling rate. We present experimental data on individual 5 nm colloidal gold nanoparticles that exhibit a near continuous density of state at 77 K. In contrast, our analysis of already published data on self-assembled InAs QDs at 4 K clearly reveals discrete degenerate energy levels.

DOI10.1021/nl504468a
Alternate JournalNano Lett.
PubMed ID25761141